Birth of the X-Ray Laser and a New Era of Science Joachim Stohr http://www-ssrl.slac.stanford.edu/stohr.

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Transcript Birth of the X-Ray Laser and a New Era of Science Joachim Stohr http://www-ssrl.slac.stanford.edu/stohr.

Birth of the X-Ray Laser and a
New Era of Science
Joachim Stohr
http://www-ssrl.slac.stanford.edu/stohr
Overview of “Light Sources”
J. Ullrich, A. Rudenko, R. Moshammer
Ann. Rev. Phys. Chem. 63, 635 (2012)
SLAC operates two world class x-ray user facilities
LCLS
SSRL storage ring
electron beam
x-ray beam
LCLS: the world’s first x-ray free electron laser
Injector
electron beam
1km linac 14GeV
AMO
SXR
Undulator hall
XPP
Near-hall: 3 stations
XCS
x-ray beam
CXI
Far-hall: 3 stations
MEC
X-Rays from SSRL
X-Ray pulse length determined by electron bunch length
Bunch width ~ 100 ps
Bunch spacing 2 ns
beam line
x-ray pulses
100 ps width/pulse
106 x-rays/pulse
500 MHz rate
Can make shorter pulses (~ 1ps) at great loss of intensity
What is a x-ray free electron laser, anyway?
Optical laser
X-ray free electron laser
10 fs width/pulse
1012 photons/pulse
120 Hz rate
• bound electrons in atoms
- transitions between discrete states
• amplification through stimulated
emission
• fixed photon energy around 1 eV
• compact size
• free electrons in bunch
- radiation in periodic H-field
• amplification through
 electron bunch orders in its own
radiation (SASE)
 electron bunch orders in imposed
radiation (seeding)
• tunable photon energy > 1000 eV
• very large size
X-Rays can see the invisible
--provide static and dynamic information--
“Imaging”
Photoemission
X-ray absorption
X-ray emission
Diffraction
EXAFS
X-ray magnetic dichroism
spin pol. photoemission
X-FEL Science
or
The Need for Speed !
The size and speed of things:
-- from “structure” to “function” --
The speed of things – the smaller the faster
macro
molecules
molecular
groups
atoms
“electrons”
& “spins”
the technology gap
optical laser pulse
Light pulses can be used to capture (or beat) all motion…
• Atoms:
Speed of sound:
1 nm / 1 ps
• Electrons:
Fermi velocity:
1 nm / 1 fs
• Light:
Speed of light:
1 nm / 3 as
Three Strategic Science Areas of LCLS
Biological structure and function Chemical structure and function
drug design, health
energy, environment
Material structure and function
information technology
Mn4CaO5 cluster
Atoms
Atoms/Electrons
Atoms/Electrons/Spins
Biological Structure: X-Rays are the key tool
(courtesy H. Chapman)
Cumulative number of structures in the PDB
ribosome
myosin
Structures
virus
nucleosome
antibody
transfer
RNA
actin
hemoglobin
myoglobin
2011
Year
C. Zardecki - PDB
C. Abad-Zapatero - Acta Cryst
D68 (2012)
Femtosecond Protein Nanocrystallography
beating the speed of sound with the speed of light
Liquid jet
atomic
structure
shape of
nanocrystal
Nanocrystals (~500nm) contained in water jet
- developed at ASU
Patterns of single nanocrystals recorded in
single, intense and fast <50 fs x-ray shots
Atoms move after shot (“speed of sound”)
crystal blows up - new crystal for new shot
Complete structure from ~1 million shots
Chemical structure: Understanding Photosynthesis
(
Water Splitting
Not Understood
)
Fixation
( Carbon
Understood )
 Has created our atmosphere and ozone layer
 Only fundamental source of food on earth

 Has created fossil energy sources (crude oil, coal, gas)
Photosystem II: Where Plants Split Water
Photosystem II
[ ]
1 ms
Mn4CaO5
X-ray damage has prevented conclusive structure determination
Beat damage with intense, fast pulses
Information Technology: Data storage
X-Rays have revealed how most advanced magnetic devices switch today
0
200ps
100 nm
SSRL
LCLS
400ps
600ps
800ps
1 ns
Tomorrow’s switching of information “bits”
Roadmap for data storage:
Magnetic “1” and “0” bits are switched by weak field pulse
aided by heat from laser
Magnetic “bits” have nanoscale dimensions
The dream: magnetic switching by a fast laser pulse
All-optical magnetic writing
Only works for one material – we do not understand process
Need LCLS: nanoscale dimension plus fast timing
LCLS is being extended by LCLS-II project
Expand capacity and capability
 New injector plus 1 km linac
 Two new undulator sources
 Extended spectral range from
250eV to 18 keV
 Experimental hall for 6 instruments
First light in fall of 2018
Assures international competitiveness
(Japan, Germany, Korea, Switzerland)