Nuclear data at n_TOF for fundamental science and technological applications Enrique M.
Download ReportTranscript Nuclear data at n_TOF for fundamental science and technological applications Enrique M.
Nuclear data at n_TOF for fundamental science and technological applications Enrique M. González Romero CIEMAT, on behalf of the n_TOF Collaboration Workshop on Applications of High Intensity Proton Accelerators Fermilab 20-X-2009 E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 1 INTRODUCTION New problems, New concepts, New materials or New procedures will need dedicated experimental validation. The first step should be done in basic experiments at specialized experimental reactors that allow to identify and separate the different Phys/Chem phenomena: E.g. Monitoring reactivity in ADS Today there are many problems where it is possible to perform high precision computer simulation. This applies in particular to neutronics, shielding and other core physics problems when nuclear data is accurate enough. In this way, simulations can optimize and enhance the value of those experiments and even reduce the number of experiments needed Today, high precision simulation is often cheaper and faster than the actual experiments, and normally provides much more details of the process – But it needs accurate basic (nuclear) data and always needs some experimental validation of its absolute accuracy. The important role of simulation and basic data is in the SRA of SNETP E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 2 Some possible (new) roles of high precision simulations include: Optimization of experiment (at any scale) planning - Significant results will be obtained? - Experimental setup/devices are appropriated - Progress vs state of the art / Conclusive results ? Exploitation (substitution) of experim. results and operational experience - Understanding available data - Interpolation of experimental results - Exploration of interest for difficult/expensive possibilities before exper. - Estimation of results for presently unreachable conditions Guiding decision making - Choices in early phases of the projects - Choices with limited (expensive) experimental information E.g. SNETP Choices of alternative systems in 2012 Education and Training Accurate nuclear data an selected basic (neutronic) experiments are key pieces to reduce uncertainties and increase confidence for safety and design E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 3 - n- induced fission (energy + wastes) - neutron capture (activation + breeding) - elastic and inelastic neutron scattering - radioactive decay - (n,xn), (n, charged particle), … Main reactions in a nuclear reactor or transmutation device (n, X+charged part.) b+ b- fission Standard reactor 1500 isotopes ADS with spallation 3000 isotopes E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 4 Rate n ( E ) ( E ) dE (E ) 238U Capture 235U Fission - n- induced fission - neutron capture - elastic and inelastic neutron scattering Thermalization, Moderation 1meV 1eV 1keV 1MeV Resonances (absorption, elastic, inelastic,…) (E ) Pressurized Water cooled Reactor (E ) Lead (Pb/Bi) cooled Fast ADS 1keV 1MeV 1meV 1eV 1keV 1MeV E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 5 Present in nuclear wastes Medium Half-Life (<100 años) Short Half-Life (< 30 dias) High A actinides Thermal and Fast Fission Fast Fissión Low Fission Cross Section TRU Transmutation Scheme Fast Spectrum Fast Spectrum Transmutation Scheme Av. Flux Intensity (n/cm2/s) 3,00E+15 Second Hour Day Year 1 Time Unit 3600 31570560 86400 3E+07 Cm242 Cm243 Cm244 Cm245 Cm246 a / SF a / EC/ SF a / SF a / SF a / SF a 100 / 6.2E-6 9 9 . 7 / 0 . 2 9 / 5 . 3 E- 9 100 / 1.35E-4 100 / 6.1E-7 100 / 3E-2 100 0,446 29,068 18,080 8490,695 4724,813 18,130 2,798 6,257 2,922 16,459 64,7% 8,0% 65,2% 11,4% 44,6% Am241 Am242 Am243 Am244 a / SF b- / EC IT / a / SF a / SF b- / EC 100 / 3.77E-10 82.7 / 17.3 9 9 . 5 / 0 . 4 6 / 1 E- 3 100 / 3.7E-9 100 / 4E-2 Am242m 432,225 0,002 140,846 3,652 7361,922 17,792 1,844 4,892 44% : 44% 13,1% 8,4% 87,0% Pu239 Pu240 Pu241 Pu242 Pu243 a / SF a / SF a / SF b- / a a / SF b- 100 / 1.9E-7 100 / 3.1E-10 100 / 5.7E-6 100 / 2.45E-3 100 / 5.5E-4 100 87,644 24083,608 6556,805 14,334 372891,707 0,001 4,220 3,477 9,033 2,688 11,354 6,775 37,5% 19,4% 54,8% 14,2% 61,1% 30,6% Np238 Np239 a / SF b- b- 100 / 2E-12 100 0,006 4,332 15,928 Pu239 a / SF 100 2137656,095 0,006 U239 <- n+U238 13,1% E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial 81,5% 15582935,494 0,001 Pu238 Np237 Cm247 Symbol & Mass Decay modes 100 / 3.1E-10 Branching ratios 24083,608 Half-Life Ln(2)/(f) 3,477 Absorption-Half-Life 19,4% (n,g)/absoption applications (AHIPA09 - Fermilab) 6 Steps to identify data needs • Identify present uncetainties • Identify relevant basic data: Isotopes, reactions, energy range Required precision for the data Priorities for different data Estimate Experimental feasibility and timely availability of experim. facilities End Users Group Designers, Builders and Utilities. Strategic choices. Simulation tools Internat. Coop/ NEA / IAEA Uncertainty evaluation (M.C., Linear Deriv.) Sensitivity analysis Global optimization and evaluation of required measurements / evaluations and needed accuracies Need for complete and reliable uncertainties and correlations. • All technologies can profit from better data: Gen II, Gen III(+), Gen IV and P&T • Industrial, Exp. Reactors and Fuel Cycle • Identify relevant parameters and target precision and priorities on those parameters Coordinate needs from different technologies/fuel cycle Reevaluation of priorities and accuracies E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 7 Fuel Fabrication (D<0.5%) Reactors: (D<0.5%) Performance: Reaction rates, Power distribution, Flux, Energy Spectrum Safety: Criticality, Feedbacks, Reactivity coeffs, Damage, Shielding Waste: Isotopic evolution, activation Nuclear Power Plant Interim Storage SPENT FUEL Storage, Reprocessing and Fabrication plants: (D<5%-10%) Reprocessing Plant High Level Wastes High Level Liquid Wastes Advanced Aqueous Partitioning Minor (MA) Actinides Fabrication of new fuels and Targets Storage, Reprocessing and Fabrication plants: (D<5%-10%) Fission (FP) Products HLW High Level Wastes Deep Geological Repository for High Level Wastes Pyrochemical Partitioning Isotopic composition !!! Radioactivity, Neutron emissions, Decay Heat, Proliferation interest ADS Transmuter Isotopic composition !!! Radioactivity, Neutron emissions, Decay Heat, Proliferation interest Radiotoxicity and Dose to Public and Environment Effective capacity Standard Advanced Reprocessing E. Gonzalez:Open Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) Cycle Reprocessing (Partitioning and Transmutation) 8 Sensitivity analysis – ADS for Transmutation keff (from G. Aliberti et al., NSE 146, 13–50, 2004) a) Upper limit of the group E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 9 NEA/WPEC-26. One possible optimization for target accuracy for innovative systems using recent covariance data evaluations (BOLNA). M. Salvatores and R. Jacqmin (Eds), NEA/WPEC-26. ISBN 978-92-64-99053-1 Similar tables for each present or proposed future reactor Still serious dependence on the reactor and fuel models and on the transmutation model (homogeneous) can slightly modify the target accuracy and details on the priority order E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 10 Important isotopes for Transmutation Fuel Cycles: The multirecycling point of view Report of the Numerical results from the Evaluation of the nuclear data sensitivities, Priority list and table of required accuracies for nuclear data. E. Gonzalez-Romero (Ed), NUDATRA Deliverable D5.11 from IP-Eurotrans T= Transmutation efficiency DH= Decay Heat load N = Neutron emission R = Radiotoxicity Isotopes 234 U U 236 U 237 Np 238 Pu 239 Pu 240 Pu 241 Pu 242 Pu 241 Am 242m Am 243 Am 242 Cm 243 Cm 244 Cm 245 Cm 246 Cm 247 Cm 248 Cm 250 Cf 252 Cf 235 Uncertainty in abundance % Burnup (GWd/t) 150 500 4.6 16.1 13.1 18.4 1.8 7.6 6.3 23.7 4.3 10.8 4.6 12.9 2.0 7.0 8.2 14.7 2.1 7.9 7.2 20.7 12.8 28.6 6.6 15.6 10.7 7.7 23.3 32.6 6.0 13.3 13.3 18.8 7.5 21.7 15.4 27.2 6.4 19.8 31.9 28.9 52.4 46.1 the Important for: 800 32.4 15.5 12.6 28.1 19.3 17.8 14.4 17.0 16.2 26.0 34.4 20.2 15.6 35.7 19.1 16.3 31.5 31.6 31.4 36.9 48.9 T T T T T T T T T T T T T DH T T T T DH DH DH DH DH DH R R R DH DH R R DH DH R N R R R N N N N E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 11 Identifying and setting priorities of Nuclear data for applications: An international endeavor • Applications set the problems to be analyzed and the required accuracies for the simulation. • Detailed uncertainty and covariance propagation to evaluate the accuracy. • Sensitivity analysis identify the relevance of each data for each isotope/reaction/energy on the most significant parameters • Linear Optimization with expert assessment of “cost” (experimental difficulties) to set priorities Efforts coordinated by dedicated expert groups of NEA/OECD, IAEA, and dedicated EU framework programs EU support and demand for nuclear data measurements: • Clear and repeated demand from the Nuclear Waste community, Sustainability of Nuclear Energy (Resources, Safety, Waste) by EU Framework Program calls: - FP5: nTOF_ND_ADS (start of n_TOF facility at CERN) - FP6: NUDATRA (inside EUROTRANS), - FP6: EFNUDAT (Transnat. Access) + CANDIDE (Roadmap for ND) - FP7: ANDES proposal to WP2009 • Collaboration with other measurements at USA, Japan, Russia. One EU call on Nuclear Data for each FP (FP5-FP7), n_TOF measurements in all of them E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 12 n_TOF Collaboration A group of 23 institutions from 14 countries (today) (A, D, Ch, Cz, E, F, I, Gr, P, Po, Ro, India, Jp, Ru) working together from 1998 to measure Precision Neutron cross sections for Nuclear Astrophysics Sustainable Nuclear Technologies Basics Physics using the neutron time of flight facility at CERN A nice social experiment of joining communities that discovered that most cross section needs and interesting measurements were common and that now share resources (shifts, detectors, analysis…) and results for each single measurement at CERN. E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 13 2000: A view of n_TOF n_TOF 185 m flight path Booster 1.4 GeV Pb Spallation Target Neutron Beam 10o prod. angle Proton Beam 20GeV/c 7x1012 ppp Linac 50 MeV PS 20GeV 2001: The real world from inside n_TOF commissioned in 2001-2002 www.cern.ch/n_TOF 2 10 1 10 0 GELINA 232 Th (0.0016 at/b) 208 Pb 10 Concept by C.Rubbia CERN/ET/Int. Note 97-19 2001-2004 Proposal submitted n-TOF 232 Th (0.0041 at/b) 208 Pb -1 10 100 1000 10000 100000 Neutron Energy / eV Phase I Isotopes Capture: 25 Fission: 11 Papers: 21 Proc.: 51 Doc: 150 Problem Investigation Phase II 2010 Construction started 10 2004-2007 Response (counts / ns) 1999 CERN/LHC/9802+Add 2009 Feasibility Aug 1998 1997 New Target construction Commissioning May 2009 2008 Commissioning TARC experiment May 1998 1995-1997 2000 n_TOF timeline Upgrades: Borated-H2O Second Line Class-A n_TOF beam characteristics • • • • • • 2nd collimator f=1.8 cm (capture mode) Wide energy range High instantaneous n- flux High resolution Low ambient background Low repetition frequency Favorable duty cycle for radioactive samples. Capture (0.1eV-1MeV) Fission (0.1 eV-20MeV) Spallation (1keV-200MeV) One of the best worldwide facilities for radioactive samples: Complementary to GELINA (EU JRC-IRMM@Geel, Belgium) E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 17 n_TOF: Advanced DAQ and detectors + Precision simulations (Geant4, MCNPX, Fluka): Utilization and Validation Low n-sensitivity capture detectors First FADC DAQ for T.o.F facilities Total Absorption Segmented Calorimeter Fission detector reconstructing F.F. trajectories E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 18 Capture 151Sm 204,206,207,208Pb, 209Bi 232Th 24,25,26Mg 90,91,92,94,96Zr, 93Zr n_TOF experiments 2000-2004 measurements Sensitivity analysis NSE 146, 13–50 (2004)) NEA/WPEC-26 (2008) 139La 186,187,188Os 233,234U NUDATRA Deliverable D5.11 of IP-Eurotrans (2009) Other types of reactor & cycles (Th-U, PWR) 237Np,240Pu,243Am Fission 233,234,235,236,238U 232Th Challenge for the first n_TOF campaign: - To improve the quality of previous measurements - Demonstrate feasibility of challenging isotopes 209Bi 237Np 241,243Am, 245Cm All data first published then stored in the EXFOR database E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 The - Fermilab) 19 n_TOF Collaboration n_TOF measurements are designed to obtain the maximum information for basic nuclear physics • Nuclear structure models - Improving the accuracy and statistical information from resolved resonances (RR) Extending the RR region Level densities and criteria for the estimation of missed resonances - Photon Strength functions from the TAC - Direct vs. compound nuclei mechanism - Measurements in closed-shell nuclei and light nuclei (Pb, Mg,…) • Fission: towards a better understanding of the process - High resolution measurements over large energy ranges in the same setup - FF kinetic energy and angular distributions determination - Fissile (233U, 235U, 245Cm) and Fissionable isotopes (234U, 232Th, …) - Sub-threshold, direct and multiple chance fission - Fine structures in the fission barriers (outer fission barrier and hyperdeformation of the fission potential) • Basic reactions - n-n scattering by 2H(n,np)n - (n, l.c.p.) reactions (l.c.p. = light charged particles like p, a, 3H, Li,…) E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 20 High resolution low backgr. of radioactive samples: 232Th by C6D6 High peak n flux intensity reduce the radioactive background + high resolution -> larger RRR + Small resonances E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 21 High resolution low backgr. of radioactive samples: 237Np TAC n_TOF capture + GELINA transmission = One of the best measur. made at Europe. C. Guerrero et al. (n_TOF Collaboration), Proc. Int. Conf. Nuc. Data for Sci. and Tech. 2007, Nice. E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 22 High resolution low capture cross section samples: C6D6 + TAC 204Pb Fitting of resonance parameter in progress! Impurities In, Sb first known Mg resonance at 20 keV 206Pb M.Heil (FZK), Nuclei in the Cosmos IX, Geneva 2005 C.Domingo-Pardo et al. (n_TOF Collaboration), Phys. Rev. C 74/75, 2006/7 E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 23 High resolution and large energy range accurate fission data 235U: High accuracy differences 245Cm: poor previous experimental results 233U: n_TOF vs ENDF BVII 238U/235U: both isotopes are fission standards up to 200 MeV. E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 24 High resolution and large energy range accurate fission data Fine structures in the fission barriers (outer fission barrier and hyper-deformation of the fission potential) E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 25 n_TOF_ph2 experiments Current program Reaching required accuracy indicated by the sensitivity analysis : (5-10%) M.A. and (2%5%) for main isotopes. Capture Stable Isotopes: Mo,Bi: Materials for fuel matrix (Mo) and coolant (Bi) Fe, Ni, Zn, 79Se: Structural materials 234,236,238U, 231Pa: Th/U fuel cycle 239,240,242Pu,241,243Am, 245Cm: transmutation of minor actinides Fission 231Pa,234,235,236,238U : Safety and sustainability of nuclear energy 241Pu,241,243Am, 244Cm, 245Cm : transmutation of minor actinides 234U: study of vibrational resonances below the barrier Other n-n scattering by 2H(n,np)n Sensitivity analysis NEA/WPEC-26 (2008) NUDATRA Deliverable D5.11 of IP-Eurotrans (2009) Other types of reactor & cycles (Th-U, PWR) (n, lcp) (lcp = light charged particles like p, a, 3H, Li,…) E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 26 n_TOF_ph2 experiments Main upgrades from n_TOF • New target, target cooling station and ventilation system (improving safety and reliability) • New fission detectors to measure more physical magnitudes (angle, kinetic energy) • New capture samples design for the calorimeter with lower beam scattered background • The possibility to have independent moderator and cooling circuits: • Moderation by borated water to reduce in-beam g background. Further upgrades ahead: • convert EAR1 to Class A/B Rad. Laboratory • Building a new short flight path and the associated experimental area EAR2 (also expected to be Class A Rad. Laboratory ) Most measurements proposed before can be done with the facility as it is (3 first upgrades), however some fission targets are conditioned by R.P. rules and will require to upgrade the Experimental Area to a Class A/B Rad. Laboratory. E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 27 The 2008 Upgrade - Design and build of new spallation target and pit lay-out - New cooling station - New ventilation system - Additional shielding and radioprotection actions - Updated detectors and DAQ New spallation target The next frontier: n_TOF @ EAR2 Present in nuclear wastes Medium Half-Life (<100 años) Short Half-Life (< 30 dias) High A actinides Thermal and Fast Fission Fast Fissión Low Fission Cross Section TRU Transmutation Scheme 238,241 242m Fast Spectrum Actinides with very short half life (10-200 yr): Pu, Am, 243,244Cm Fast Spectrum Transmutation Scheme Av. Flux Intensity (n/cm2/s) 3,00E+15 Second Hour Day Year 1 Time Unit 3600 31570560 86400 3E+07 Cm242 Cm243 Cm244 Cm245 Cm246 a / SF a / EC/ SF a / SF a / SF a / SF a 100 / 6.2E-6 9 9 . 7 / 0 . 2 9 / 5 . 3 E- 9 100 / 1.35E-4 100 / 6.1E-7 100 / 3E-2 100 0,446 29,068 18,080 8490,695 4724,813 18,130 2,798 6,257 2,922 16,459 64,7% 8,0% 65,2% 11,4% 44,6% Am241 Am242 Am243 Am244 a / SF b- / EC IT / a / SF a / SF b- / EC 100 / 3.77E-10 82.7 / 17.3 9 9 . 5 / 0 . 4 6 / 1 E- 3 100 / 3.7E-9 100 / 4E-2 Am242m 432,225 0,002 140,846 7361,922 3,652 17,792 1,844 4,892 44% : 44% 13,1% 8,4% 87,0% Pu239 Pu240 Pu241 Pu242 Pu243 a / SF a / SF a / SF b- / a a / SF b- 100 / 1.9E-7 100 / 3.1E-10 100 / 5.7E-6 100 / 2.45E-3 100 / 5.5E-4 100 24083,608 6556,805 14,334 372891,707 0,001 4,220 3,477 9,033 2,688 11,354 6,775 37,5% 19,4% 54,8% 14,2% 61,1% 30,6% Np237 Np238 Np239 a / SF b- b- a / SF 100 / 2E-12 100 100 100 / 3.1E-10 2137656,095 0,006 4,332 15,928 81,5% 13,1% 0,006 15582935,494 0,001 Pu238 87,644 Cm247 Pu239 Ln(2)/(f) 24083,608 3,477 19,4% Symbol & Mass Decay modes Branching ratios Half-Life Absorption-Half-Life (n,g)/absoption • These isotopes are key steps for the nuclear waste breeding, but their radioactivity makes their measurement very difficult. • Very low mass samples (<<1 mg): to reduce the radioactivity induced background and to be compatible with R.P. rules. • Same conditions allow very rare materials (even deposits from rad beams ISOLDE?), and materials of very low cross section: 90Sr, 79Se, 126Sn, 147Pm, 135Cs: long lived FF E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 29 The next frontier: n_TOF @ EAR2 (1) (2) (3) (4) (5) Radioactivity background High brightness (peak flux intensity) and low duty cycle Shorter flight path 1/10 -> 10-100 times larger flux (EAR2) Scattered beam background Very thin sample support no encapsulation Class A laboratory (EAR2) Distance from samples to walls (EAR2) Background vs. Detectors Low neutron sensitivity of detectors Improved background rejection by detectors In beam background Large angle of neutron and proton lines (EAR2) Optimized moderator Ambient background Walls distance and detector background rejection New experimental area at 20 m n_TOF target Experimental area at 185 m E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 30 Summary and conclusions • n_TOF @ CERN is a first class neutron Time Of Flight facility • It is specially well suited for radioactive materials, samples of rare materials or low cross section. • Excellent facility for measuring neutron capture and fission cross sections and the most needed cross sections identified for nuclear applications (nuclear waste minimization). Sustained support from the EU framework programs. • The measurements provide very relevant parameters to improve the understanding and physics models of nuclides and reactions. • Combined with high performance detectors and DAQ allows to perform high accuracy cross section measurements. • The n_TOF potentiality was proved by successful operation from 2000 to 2004 • The current campaign, with improved setup, will allow to fully exploit its possibilities to fulfill the request of the highest priority nuclear data needs • There are plans to enhance the performance with an additional short flight path and EAR2 that will allow to open a new frontier of sample masses, short lived isotopes and accurate measurements E. Gonzalez: Nuclear data at n_TOF for fundamental science and industrial applications (AHIPA09 - Fermilab) 31