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Quantum Effects in BECs and FELs Nicola Piovella, Dipartimento di Fisica and INFN-Milano Rodolfo Bonifacio, INFN-Milano Luca Volpe (PhD student), Dipartimento di Fisica-Milano Mary Cola (Post Doc), Dipartimento di Fisica-Milano Gordon R. M. Robb, University of Strathclyde, Glasgow, Scotland. work supported by INFN (QFEL project) Outline 1. Introductory concepts 2. Classical FEL-CARL Model 3. Quantum FEL-CARL Model 4. Propagation Effects 5. Quantum SASE regime Free Electron Laser (FEL) w r 2 2 Collective Atomic Recoli Laser (CARL) Pump beam wp R. Bonifacio et al, Opt. Comm. 115, 505 (1995) Probe beam w wp Both FEL and CARL are examples of collective recoil lasing Pump field CARL ~p Cold atoms Backscattered field (probe) SN SNSN FEL Electron beam N S N SN S “wiggler” magnet (period w) EM radiation w /2 << w At first sight, CARL and FEL look very different… Connection between CARL and FEL can be seen more easily by transforming to a frame (L’) moving with electrons FEL electrons EM pump, ’w (wiggler) Backscattered EM field ’ ’w CARL Pump laser Connection between FEL and CARL is now clear Cold atoms Backscattered field ~p In FEL and CARL particles self-organize to form compact bunches ~ which radiate coherently. Collective Recoil Lasing = Optical gain + bunching bunching factor b (0<|b|<1): 1 b N N e j 1 i j Exponential growth of the emitted radiation: Both FEL and CARL are described using the same ‘classical’ equations, but different independent variables. j FEL: 2 ( Ae i j z A A 1 z z1 N 2 c.c.) N e i j (k kw ) z wt ; iA j 1 CARL: 2kz ; z wrec t z1 wrec ( z / c) 1/ 3 2k 2 PL n1/ 3 wrec 2/3 m a z1 z v 0t Lc w Lg ; 4 z z Lg Lc Lg ; w mc 0 Bw 2 / 3n1/ 3 k | A| 2 N photons N CARL-FEL instability animation A 0 z1 Animation shows evolution of electron/atom positions in the dynamic pendulum potential together with the probe field intensity. V ( ) 2 | A | cos( ) Linear Theory (classical) Ae iz 2 1 0 runaway solution wp w mc( 0 r ) ( FEL) (CARL) k wrec See figure (a) Maximum gain at =0 | A| e 2 3z Quantum model of FEL/CARL We now describe electrons/atoms as QM wavepackets, rather than classical particles. Procedure : Describe N particle system as a Q.M. ensemble Write Schrodinger equation for macroscopic wavefunction ( , z ) Include propagation using a multiple-scaling approach ( , z , z1 ) Canonical Quantization p H p H p Ae c.c. i pz m c( 0 ) p ( FEL ) k k p2 H i Aei c.c. 2 so Quantization (with classical field A) : p pˆ i so [ˆ, pˆ ] i H Hˆ ˆ i H z 1 2 i i i A ( z ) e c.c. 2 z 2 dA dz 2 d ( , z ) e i iA 2 0 R. Bonifacio, N. Piovella, G.R.M.Robb and M.Cola, Optics Comm, 252, 381 (2005) Quantum FEL Propagation model So far we have neglected slippage, so all sections of the e-beam evolve identically (steady-state regime) if they are the same initially. We have introduced propagation into the model, so different parts of the electron beam can feel different fields : i 2 i [ A ( z , z ) e c.c.] 1 2 z 2 A A z z1 2 d ( , z , z1 ) 2 e i iA 0 Here describes spatial evolution of on scale of and z1 describes spatial evolution of A and on scale of cooperation length, Lc >> . z1 ( z vr t ) / Lc where Lc 4 Quantum Dynamics 0,2 ( , z , z1 ) cn ( z , z1 )ein n ein is momentum eigenstate corresponding to eigenvalue Only discrete changes of momentum are possible : pz n=1 n=0 n=-1 n( k ) pz= n (k) , n=0,±1,.. k cn in 2 cn Acn 1 A*cn 1 z 2 A A cn cn*1 iA z z1 n | cn |2 pn probability to find a particle with p=n(ħk) =10, no propagation A 0 z1 1 steady-state evolution: 10 (a) -1 10 -3 |A| classical limit is recovered for 2 10 -5 10 -7 10 -9 1 10 0 10 20 30 40 50 z 0.15 (b) pn many momentum states occupied, both with n>0 and n<0 0.10 0.05 0.00 -15 -10 -5 0 n 5 10 Quantum limit for 1 A 0 z 1 Only TWO momentum states involved : n=0 and n= - 1 ( , z ) c0 ( z ) c1 ( z )ei n=0 n=-1 Dynamics are those of a 2-level system coupled to an optical field,described by Maxwell-Bloch equations 0.1 0.0 10 -0.2 8 2 |A| -0.4 6 <p> 4 -0.6 2 -0.8 0 0 100 200 z -1.0 0 100 200 z Bunching and density grating QUANTUM REGIME <1 CLASSICAL REGIME >>1 0.6 0.15 0.5 0.4 pn pn 0.10 0.3 0.2 0.05 0.1 0.00 -20 -15 -10 -5 0 5 10 -5 -4 -3 -2 -1 15 10 2.0 | ( ) |2 8 | ( ) |21.5 6 N( )/N N( )/N 1 2 3 4 5 n n 4 1.0 0.5 2 0 0 0.0 0 1 2 3 /2 4 5 0 ( ) cn ein n 1 2 3 /2 4 5 A e iz Quantum Linear Theory 2 1 2 1 0 4 1 Quantum regime for <1 1.0 0.8 Classical limit |Im| 0.6 (a) (a) 2 (b) 2. (c) 2 (d) 2 (e) 2 (f) 2 (b) 1 max at 2 m c( 0 r ) k / 2 ( FEL) w w w (CARL) p rec (c) 0.4 (d) (e) (f) 0.2 0.0 -10 2 1 0 width -5 0 5 10 15 QUANTUM CARL HAS BEEN OBSERVED WITH BECs IN SUPERRADIANT REGIME (MIT, LENS) When the light escapes rapidly from the sample of length L, we see a sequential Super-Radiant (SR) scattering, with atoms recoiling by 2ħk, each time emitting a SR pulse 2 dcn in * cn Acn 1 A cn 1 dz 2 dA * cn cn 1 iA KA dz n damping of radiation c K L SEQUENTIAL SUPERRADIANT SCATTERING LASER n=0 BEC 2k n=-1 n=-2 | A |2 N 2 sec h2 ( gNz) 0 2k 0.002 2 |A| <p> -2 0.001 -4 0.000 0 250 500 z 0 250 500 z Superradiant Rayleigh Scattering in a BEC (Ketterle, MIT 1991) for K>>1 and K Experimental evidence of quantum CARL at LENS • Production of an elongated 87Rb BEC in a magnetic trap • Laser pulse during first expansion of the condensate • Absorption imaging of the momentum components of the cloud trap BEC g laser beam w, k Experimental values: = 13 GHz w = 750 mm P = 13 mW absorption imaging p 2 k L.Fallani et al, PRA 71 (2005) 033612 The experiment Temporal evolution of the population in the first three atomic momentum states during the application of the light pulse. pump light n=0 (p=0) n=-2 n=-1 (p=2ħk) (p=4ħk) PROPAGATION EFFECTS IN FELs : SUPERRADIANT INSTABILITY Particles at the trailing edge of the beam never receive radiation from particles behind them: they just radiate in a SUPERRADIANT PULSE or SPIKE which propagates forward. if Lb << Lc the SR pulse remains small (weak SR). if Lb >> Lc the weak SR pulse gets amplified (strong SR) as it propagates forward through beam with no saturation. The SR pulse is a self-similar solution of the propagation equation. SR in the classical model: A A ei z z1 Strong SR (Lb=30 Lc) from a coherent seed z vt z1 Lc R. Bonifacio, B.W. McNeil, and P. Pierini PRA 40, 4467 (1989) CLASSICAL SASE Ingredients of Self Amplified Spontaneous Emission (SASE) i) Start up from noise ii) Propagation effects (slippage) iii) SR instability The electron bunch behaves as if each cooperation length would radiate independently a SR spike which is amplified propagating on the other electrons without saturating. Spiky time structure and spectrum. SASE is the basic method for producing coherent X-ray radiation in a FEL CLASSICAL SASE Time profile with many random spikes (approximately L/Lc) Broad and noisy spectrum at short wavelengths (X-FEL) Example from DESY (Hamburg) for the SASE-FEL experiment SASE : NUMERICAL SIMULATIONS L 30Lc CLASSICAL REGIME: 5 QUANTUM REGIME: 0.1 SASE: average momentum distribution CLASSICAL REGIME: 5 Classical behaviour : both n<0 and n>0 occupied QUANTUM REGIME: 0.1 Quantum behaviour : sequential SR decay, only n<0 0.1 1/ 10 0.3 1/ 3.3 0.2 1/ 5 0.4 1/ 2.5 Quantum SASE: Spectral purification and multiple line spectrum • In the quantum regime the gain bandwidth 3/ 2 decreases as 4 line narrowing. • Spectrum with multiple lines. When the width of each line becomes larger or equal to the line separation, continuous spectrum, i.e., classical limit. This happens when 4 3/ 2 1 0.4 FEL IN SASE REGIME IS ONE OF THE BEST CANDIDATE FOR AN X-RAY SOURCE (=1Ǻ) CLASSICAL SASE needs: GeV Linac (Km) Long undulator (100 m) High cost (109 $) yields: Broad and chaotic spectrum QUANTUM SASE needs: MeV Linac (m) Laser undulator (~1mm) lower cost (106 $) yields: quasi monocromatic spectrum CONCLUSIONS • Classical FEL/CARL model - classical motion of electrons/atoms - continuous momenta • Quantum FEL/CARL model - QM matter wave in a self consistent field - discrete momentum state and line spectrum • Quantum model with propagation - new regime of SASE with quantum ”purification’’ - appearance of multiple narrow lines