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Negative refraction and Left-handed behavior in Photonic Crystals: FDTD and Transfer matrix method studies Peter Markos, S. Foteinopoulou and C. M. Soukoulis Outline of Talk • • • • What are metamaterials? Historical review Left-handed Materials Results of the transfer matrix method Determination of the effective refractive index • Negative n and FDTD results in PBGs (ENE & SF) • New left-handed structures • Experiments on negative refractions (Bilkent) • Applications/Closing Remarks E. N. Economou & S. Foteinopoulou What is an Electromagnetic Metamaterial? A composite or structured material that exhibits properties not found in naturally occurring materials or compounds. Left-handed materials have electromagnetic properties that are distinct from any known material, and hence are examples of metamaterials. Electromagnetic Metamaterials Example: Metamaterials based on repeated cells… Veselago We are interested in how waves propagate through various media, so we consider solutions to the wave equation. E 2 E em 2 t 2 e,m space (-,+) k em (-,-) n em (+,+) (+,-) Sov. Phys. Usp. 10, 509 (1968) Left-Handed Waves • If e 0, m 0 then vectors: • If e 0, m 0 then vectors: E, H , k is a right set of is a left set of E, H , k Energy flux in plane waves • Energy flux (Pointing vector): – Conventional (right-handed) medium – Left-handed medium Frequency dispersion of LH medium • Energy density in the dispersive medium e 2 m 2 W E H • Energy density W must be positive and this requires e 0; • LH medium is always dispersive m 0 • According to the Kramers-Kronig relations – it is always dissipative “Reversal” of Snell’s Law PIM RHM PIM RHM PIM RHM NIM LHM 2 1 (1) 2 1 (2) k S (1) (2) k S Focusing in a Left-Handed Medium RH RH RH RH LH RH n=1 n=1.3 n=1 n=1 n=-1 n=1 PBGs as Negative Index Materials (NIM) Veselago : Materials (if any) with e < 0 and m< 0 em>0 Propagation k, E, H Left Handed (LHM) S=c(E x H)/4p opposite to k Snell’s law with g opposite to k n em Flat lenses Super lenses < 0 (NIM) Objections to the left-handed ideas Parallel momentum is not conserved S1 S2 A Causality is violated Fermat’s Principle Superlensing is not possible O΄ B Μ Ο ndl minimum (?) Reply to the objections • Photonic crystals have practically zero absorption • Momentum conservation is not violated • Fermat’s principle is OK ndlextremum • Causality is not violated • Superlensing possible but limited to a cutoff kc or 1/L Materials with e < 0 and m<0 g opposite to k S u g S opposite to k 1 S opposite to k dn n d n 0 c p g , p k0 n m k 2 m 2 p 2 S E H c 8p u p k Photonic Crystals g opposite to k S u g 1 dn n d n n 0 n n , , 0 , 0 p c g , p k0 n ck Super lenses 2 c 2k||2 k2 if k|| /c k is imaginary e ik r ~e k r Wave components with decay, i.e. are lost , then Dmax l If n < 0, phase changes sign k k || e ik r ~e k r thus k if k imaginary k| | / c ARE NOT LOST !!! Metamaterials Extend Properties 2p e 1 2 J. B. Pendry 2p m 1 2 02 First Left-Handed Test Structure UCSD, PRL 84, 4184 (2000) Transmitted Power (dBm) Transmission Measurements Wires alone Split rings alone m>0 e<0 m<0 e<0 m>0 e<0 e<0 Wires alone 4.5 5.0 5.5 6.0 Frequency (GHz) 6.5 7.0 UCSD, PRL 84, 4184 (2000) A 2-D Isotropic Structure UCSD, APL 78, 489 (2001) Measurement of Refractive Index UCSD, Science 292, 77 2001 Measurement of Refractive Index UCSD, Science 292, 77 2001 Measurement of Refractive Index UCSD, Science 292, 77 2001 Transfer matrix is able to find: • Transmission (p--->p, p--->s,…) p polarization • Reflection (p--->p, p--->s,…) s polarization • Both amplitude and phase • Absorption Some technical details: • Discretization: unit cell Nx x Ny x Nz : up to 24 x 24 x 24 • Length of the sample: up to 300 unit cells • Periodic boundaries in the transverse direction • Can treat 2d and 3d systems • Can treat oblique angles • Weak point: Technique requires uniform discretization Structure of the unit cell EM wave propagates in the z -direction Periodic boundary conditions are used in transverse directions Polarization: p wave: E parallel to y s wave: E parallel to x For the p wave, the resonance frequency interval exists, where with Re meff <0, Re eeff<0 and Re np <0. For the s wave, the refraction index ns = 1. Typical size of the unit cell: 3.3 x 3.67 x 3.67 mm Typical permittivity of the metallic components: emetal = (-3+5.88 i) x 105 Structure of the unit cell: SRR EM waves propagate in the z-direction. Periodic boundary conditions are used in the xy-plane LHM Left-handed material: array of SRRs and wires Resonance frequency as a function of metallic permittivity complex em Real em Dependence of LHM peak on metallic permittivity The length of the system is 10 unit cells Dependence of LHM peak on metallic permittivity PRB 65, 033401 (2002) Example of Utility of Metamaterial exp(ikd) ts 1 1 cosnkd z sinnkd 2 z The transmission coefficient is an example of a quantity that can be determined simply and analytically, if the bulk material parameters are known. z rs ts exp(ikd)i(z 1 / z)sin(nkd ) / 2 UCSD and ISU, PRB, 65, 195103 (2002) m e n me 2ep e 1 2 2e0 ie 0 2mp m 1 2 2m0 im0 Effective permittivity e and permeability m of wires and SRRs UCSD and ISU, PRB, 65, 195103 (2002) Effective permittivity e and permeability m of LHM UCSD and ISU, PRB, 65, 195103 (2002) Effective refractive index n of LHM UCSD and ISU, PRB, 65, 195103 (2002) Determination of effective parameters from transmission studies From transmission and reflection data, the index of refraction n was calculated. Frequency interval with Re n<0 and very small Im n was found. Pe rm ittivitye, Pe rm e abilitym and Im pe danceZ Re m < 0 Re e < 0 Im m> 0 Im e < 0 ??? Im Z < 0 Re > 0 Energy lossesQ are always positive in spite of the fact thatIm e is negative: Q()= 2/(2p) |H|2 Im (n) Re (Z) > 0 Another 1D left-handed structure: Both SRR and wires are located on the same side of the dielectric board. Transmission depends on the orientation of SRR. Bilkent & ISU APL 2002 0.33 mm w t»w t t=0.5 or 1 mm w=0.01 mm 0.33 mm l=9 cm 3 mm 0.33 mm 3 mm ax Periodicity: ax=5 or 6.5 mm ay=3.63 mm az=5 mm Polarization: TM y E x B y z x Number of SRR Nx=20 Ny=25 Nz=25 New designs for left-handed materials eb=4.4 Bilkent and ISU, APL 81, 120 (2002) ax=6.5 mm t= 0.5 mm Transmission (dB) 0 -10 -20 -30 SRR Wire LHM -40 -50 -60 7 8 9 10 11 12 13 Frequency (GHz) Bilkent & ISU APL 2002 14 ax=6.5 mm t= 1 mm Transmission (dB) 0 SRR Wire LHM -10 -20 -30 -40 -50 -60 7 8 9 10 11 12 13 Frequency (GHz) Bilkent & ISU APL 2002 14 Cut wires: Positive and negative n Phase and group refractive index •In both the LHM and PC literature there is still a lot of confusion regarding the phase refractive index np and the group refractive index ng. How these properties relate to “negative refraction” and LH behavior has not yet been fully examined. •There is controversy over the “negative refraction” phenomenon. There has been debate over the allowed signs (+ /-) for np and ng in the LH system. DEFINING phase and group refractive index np and ng In any general case: The equifrequency surfaces (EFS) (i.e. contours of constant frequency in 2D k-space) in air and in the PC are needed to find the refracted wavevector kf (see figure). vphase=c/|np| and vgroup= k c/|ng| Where c is the velocity of light So from k// momentum conservation: |np|=c kf () /. Remarks In the PC system vgroup=venergy so |ng|>1. Indeed this holds ! np <1 in many cases, i.e. the phase velocity is larger than c in many cases. np can be used in Snell’s formula to determine the angle of the propagating wavevector. In general this angle is not the propagation angle of the signal. This angle is the propagation angle of the signal only when dispersion is linear (normal), i.e. the EFS in the PC is circular (i.e. kf independent of theta). ng can never be used in a Snell-like formula to determine the signals propagation angle. Index of refraction of photonic crystals – The wavelength is comparable with the period of the photonic crystal – An effective medium approximation is not valid ky Effective index kx Refraction angle Equifrequency surfaces Incident angle Photonic Crystals with negative refraction. Photonic Crystals with negative refraction. S. Foteinopoulou, E. N. Economou and C. M. Soukoulis Schematics for Refraction at the PC interface EFS plot of frequency a/l = 0.58 Schematics for Refraction at the PC interface EFS plot of frequency a/l = 0.535 Negative refraction and left-handed behavior for a/l = 0.58 Negative refraction but NO left-handed behavior for a/l = 0.535 Superlensing in 2D Photonic Crystals Lattice constant=4.794 mm Dielectric constant=9.73 r/a=0.34, square lattice Experiment by Ozbay’s group Negative Refraction in a 2d Photonic Crystal Band structure, negative refraction and experimental set up Frequency=13.7 GHz Negative refraction is achievable in this frequency range for certain angles of incidence. Bilkent & ISU Superlensing in photonic crystals Subwavelength Resolution in PC based Superlens The separation between the two point sources is l/3 Photonic Crystals with negative refraction. Photonic Crystal vacuum FDTD simulations were used to study the time evolution of an EM wave as it hits the interface vacuum/photonic crystal. Photonic crystal consists of an hexagonal lattice of dielectric rods with e=12.96. The radius of rods is r=0.35a. a is the lattice constant. Photonic Crystals with negative refraction. t0=1.5T T=l/c Photonic Crystals with negative refraction. Photonic Crystals with negative refraction. Photonic Crystals with negative refraction. Photonic Crystals: negative refraction The EM wave is trapped temporarily at the interface and after a long time, the wave front moves eventually in the negative direction. Negative refraction was observed for wavelength of the EM wave l= 1.64 – 1.75 a (a is the lattice constant of PC) Conclusions • Simulated various structures of SRRs & LHMs • Calculated transmission, reflection and absorption • Calculated meff and eeff and refraction index (with UCSD) • Suggested new designs for left-handed materials • Found negative refraction in photonic crystals • A transient time is needed for the wave to move along the - direction • Causality and speed of light is not violated. • Existence of negative refraction does not guarantee the existence of negative n and so LH behavior • Experimental demonstration of negative refraction and superlensing • Image of two points sources can be resolved by a distance of l/3!!! $$$ DOE, DARPA, NSF, NATO, EU Publications: P. Markos and C. M. Soukoulis, Phys. Rev. B 65, 033401 (2002) P. Markos and C. M. Soukoulis, Phys. Rev. E 65, 036622 (2002) D. R. Smith, S. Schultz, P. Markos and C. M. Soukoulis, Phys. Rev. B 65, 195104 (2002) M. Bayindir, K. Aydin, E. Ozbay, P. Markos and C. M. Soukoulis, Appl. Phys. Lett. (2002) P. Markos, I. Rousochatzakis and C. M. Soukoulis, Phys. Rev. E 66, 045601 (R) (2002) S. Foteinopoulou, E. N. Economou and C. M. Soukoulis, PRL, accepted (2003) S. Foteinopoulou and C. M. Soukoulis, submitted Phys. Rev. B (2002) P. Markos and C. M. Soukoulis, submitted to Opt. Lett. E. Cubukcu, K. Aydin, E. Ozbay, S. Foteinopoulou and C. M. Soukoulis, submitted to Nature P. Markos and C. M. Soukoulis, submitted to Optics Express The keen interest to the topic 40 30 20 10 0 1968 1980 1990 1996 1999 2001 • Terminology • • • • • • Left-Handed Medium (LH) Metamaterial Backward Medium (BW) Double Negative Medium (DNG) Negative Phase Velocity (NPV) Materials with Negative Refraction (MNR) Collaboration between Crete, Greece and Bilkent University, Turkey Crete GM Image Plane Experimental Setup Network Analyzer Scanned Power Distribution at the Image Plane 13.698 GHz Average Intensity 1.0 Experiment Theory 0.8 0.6 0.4 0.2 0.0 -5 -4 -3 -2 -1 0 1 Detuning (cm) 2 3 4 5 Dependence of LHM peak on L and Im em Dependence on the incident angle Transmission peak does not depend on the angle of incidence ! This structure has an additional xz - plane of symmetry Transition peak strongly depends on the angle of incidence. Transmission depends on the orientation of SRR Transmission properties depend on the orientation of the SRR: Lower transmission Narrower resonance interval Lower resonance frequency Higher transmission Broader resonance interval Higher resonance frequency Dependence of the LHM T peak on the Im eBoard In our simulations, we have: Periodic boundary condition, therefore no losses due to scattering into another direction. Very high Im emetal therefore very small losses in the metallic components. Losses in the dielectric board are crucial for the transmission properties of the LH structures. New / Alternate Designs Superprism Phenomena in Photonic Crystals Experiment – H.Kosaka, T.Kawashima et. al. Superprism phenomena in photonic crystals, Phys. Rev. B 58, 10096 (1998) Scattering of the photonic crystal Hexagonal 2D photonic crystal -M.Natomi, Phys. Rev. B 62, 10696 (2000) Using an equifrequency surface (EFS) plots Vanishingly small index modulation Small index modulation Photonic crystal as a perfect lens C. Luo, S. G. Johnson, J. D. Joannopoulos, and J. B. Pendry Phys. Rev. B, 65, 201104 (2002) Resolution limit 0.67 l