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The origin of heavy elements in the solar system (Pagel, Fig 6.8) each process contribution is a mix of many events ! 1 Abundance pattern: “Finger print” of the r-process ? Tellurium and Xenon Peak Abundance (Si = 106) Solar abundance of the elements Platinum Peak r-process only (subtract s,p processes) Element number (Z) But: sun formed ~10 billion years after big bang: many stars contributed to elements This could be an accidental combination of many different “fingerprints” ? Find a star that is much older than the sun to find “fingerprint” of single event 2 Heavy elements in Metal Poor Halo Stars recall: [X/Y]=log(X/Y)-log(X/Y)solar CS22892-052 red (K) giant located in halo distance: 4.7 kpc mass ~0.8 M_sol [Fe/H]= -3.0 [Dy/Fe]= +1.7 old stars - formed before Galaxy was mixed they preserve local pollution from individual nucleosynthesis events 3 A single (or a few) r-process event(s) CS22892-052 (Sneden et al. 2003) 1 solar r Cosmo Chronometer 0 -1 -2 40 NEW: CS31082-001 with U (Cayrel et al. 2001) 50 other, second r-process to fill this up ? (weak r-process) 60 70 80 element number main r-process matches exactly solar r-pattern conclusions ? 90 Age: 16+- 3 Gyr (Schatz et al. 2002 ApJ 579, 626) 4 New Observations r-process elements from single r-process events in 3 very metal poor stars Solar r-process elements from many events J. Cowan Many more to come from ongoing surveys and followup campaigns (e.g. VLT) 5 Overview heavy element nucleosynthesis process conditions timescale site s-process (n-capture, ...) T~ 0.1 GK tn~ 1-1000 yr, nn~107-8/cm3 102 yr and 105-6 yrs Massive stars (weak) Low mass AGB stars (main) r-process (n-capture, ...) T~1-2 GK tn ~ ms, nn~1024 /cm3 < 1s Type II Supernovae ? Neutron Star Mergers ? p-process ((g,n), ...) T~2-3 GK ~1s Type II Supernovae Light Element Primary Process (LEPP) ? ? (maybe s-process like?) ? (long if sprocess) ? 6 The r-process Temperature: ~1-2 GK Density: 300 g/cm3 (~60% neutrons !) Rapid neutron capture neutron capture timescale: ~ 0.2 ms b-decay Seed (g,n) photodisintegration Equilibrium favors “waiting point” Neutron number 7 Waiting point approximation Definition: ASSUME (n,g)-(g,n) equilibrium within isotopic chain How good is the approximation ? This is a valid assumption during most of the r-process BUT: freezeout is neglected Freiburghaus et al. ApJ 516 (2999) 381 showed agreement with dynamical models Consequences During (n,g)-(g,n) equilibrium abundances within an isotopic chain are given by: Y ( Z , A 1) G ( Z , A 1) A 1 2 nn Y ( Z , A) 2G ( Z , A) A mu kT 2 3/ 2 exp(S n / kT ) • time independent • can treat whole chain as a single nucleus in network • only slow beta decays need to be calculated dynamically • neutron capture rate independent (therefore: during most of the r-process n-capture rates do not matter !) 8 Pt Xe Ni 78Ni, 79Cu first bottle necks in n-capture flow (80Zn later) 79Cu: half-life measured 188 ms (Kratz et al, 1991) 78Ni : half-life predicted 130 – 480 ms 2 events @ GSI (Bernas et al. 1997) 9 H. Schatz Nuclear physics in the r-process b-delayed n-emission branchings (final abundances) Fission rates and distributions: • n-induced • spontaneous • b-delayed b-decay half-lives (abundances and process speed) n-capture rates • in slow freezeout • maybe in a “weak” r-process ? n-phyiscs ? Seed production rates (aaa,aan, a2n, ..) Masses (Sn) (location of the path) 10 Sensitivity of r-process to astro and nuclear physics Sensitivity to astrophysics Sensitivity to nuclear physics 1 Abundance Hot bubble Classical model Same nuclear physics 10 ETFSI-Q masses ETFSI-1 masses Same r-process model 0 10 -1 10 -2 10 -3 10 Freiburghaus et al. 1999 -4 10 Mass number Contains information about: • n-density, T, time (fission signatures) • freezeout • neutrino presence • which model is correct 100 120 140 160 180 200 220 Mass number But convoluted with nuclear physics: • masses (set path) • T1/2, Pn (Y ~ T1/2(prog), key waiting points set timescale) • n-capture rates • fission barriers and fragments 11 Shell quenching effect on masses/r-process Ru Pd Cd S2n (MeV) Mo Zr r-process path ETFSI-1 Neutron number 12 Shell quenching effect on masses/r-process Ru Pd Cd Mo Zr S2n (MeV) distinguish ETFSI-1 ETFSI-Q (N=82 quenched) Neutron number 13 Endpoint of the r-process r-process ended by n-induced fission or spontaneous fission (different paths for different conditions) (Goriely & Clerbaux A&A 348 (1999), 798 n-induced fission (Z,A) n-capture (DC) fission (Z,A+1) b-delayed fission (Z,A) spontaneous fission bfission (Z+1,A) (Z,A+1) fission barrier fission 14 Consequences of fission Fission produces A~Aend/2 ~ 125 nuclei modification of abundances around A=130 peak fission products can serve as seed for the r-process - are processed again into A~250 region via r-process - fission again fission cycling ! Note: the exact endpoint of the r-process and the degree and impact of fission are unknown because: • Site conditions not known – is n/seed ratio large enough to reach fission ? (or even large enough for fission cycling ?) • Fission barriers highly uncertain • Fission fragment distributions not reliably calculated so far (for fission from excited states !) 15 Role of beta delayed neutron emission Neutron rich nuclei can emit one or more neutrons during b-decay if Sn<Qb (the more neutron rich, the lower Sn and the higher Qb) (Z,A) bn Sn g (Z+1,A-1) (Z+1,A) If some fraction of decay goes above Sn in daughter nucleus then some fraction Pn of the decays will emit a neutron (in addition to e- and n) (generally, neutron emission competes favorably with g-decay - strong interaction !) 16 Effects: during r-process: none as neutrons get recaptured quickly during freezeout • modification : of final abundance • late time neutron production (those get recaptured) Calculated r-process production of elements (Kratz et al. ApJ 403 (1993) 216): before b-decay after b-decay smoothing effect from b-delayed n emission ! 17 Cs (55) Cs131 Cs132 Cs133 Cs134 Cs135 Cs136 Cs137 Cs138 Cs139 Cs140 Cs141 Cs142 Cs143 Cs144 Cs145 Cs146 Cs147 > 99 Xe (54) I (53) Te (52) Sb (51) Sn (50) In (49) Cd (48) Ag (47) > 99 > 99 19.00 > 99 > 99 > 99 63.70 24.94 1.70 1.78 1.01 0.59 0.32 0.23 Xe130 Xe131 Xe132 Xe133 Xe134 Xe135 Xe136 Xe137 Xe138 Xe139 Xe140 Xe141 Xe142 Xe143 Xe144 Xe145 Xe146 > 99 I129 > 99 Pn39.68 =0% 13.60 > 99 > 99 I137 1.73 1.24 0.30 1.15 0.90 I142 I143 I144 I130 I131 I132 I133 I134 I135 I136 I138 I139 I140 I141 > 99 > 99 > 99 > 99 > 99 > 99 83.40 24.50 6.49 2.28 0.86 0.43 I145 r-process waiting point Te128 Te129 Te130 Te131 Te132 Te133 Te134 Te135 Te136 Te137 Te138 Te139 Te140 Te141 Te142 Te143 Te144 > 99 > 99 > 99 > 99 > 99 19.00 17.50 2.49 P =99.9% 1.40 n Sb134 Sb135 Sb136 Sb137 Sb138 Sb139 Sb140 Sb141 Sb142 Sb143 Sb127 Sb128 Sb129 Sb130 Sb131 Sb132 Sb133 > 99 > 99 > 99 > 99 > 99 > 99 > 99 1.66 0.82 Sn126 Sn127 Sn128 Sn129 Sn130 Sn131 Sn132 Sn133 Sn134 Sn135 Sn136 Sn137 Sn138 Sn139 Sn140 Sn141 Sn142 > 99 > 99 > 99 > 99 > 99 56.00 39.70 1.20 1.12 In125 In126 In127 In128 In129 In130 In131 In132 In133 In134 In135 In136 In137 In138 In139 In140 In141 2.36 1.60 1.09 0.84 0.61 0.26 0.28 0.20 Example: impact of Pn for 137Sb Cd138 Cd139 Cd140 0.18 Cd124 Cd125 Cd126 Cd127 Cd128 Cd129 Cd130 Cd131 Cd132 Cd133 Cd134 Cd135 Cd136 1.24 0.65 0.51 0.43 0.34 0.27 0.20 A=136 ( 99%) Ag123 Ag124 Ag125 Ag126 Ag127 Ag128 Ag129 Ag130 Ag131 Ag132 Ag133 0.29 0.17 0.16 0.10 0.11 0.06 0.05 76 77 78 79 80 81 82 83 84 85 86 A=137 ( 0%) Ag135 Ag136 Ag137 Ag138 Ag139 87 88 89 90 91 92 r-process waiting point 18 Summary: Nuclear physics in the r-process Quantity Effect Sn neutron separation energy path T1/2 b-decay half-lives • abundance pattern • timescale Pn b-delayed n-emission branchings final abundance pattern • endpoint • abundance pattern? • degree of fission cycling fission (branchings and products) G partition functions • path (very weakly) NA<sv> neutron capture rates • final abundance pattern during freezeout ? • conditions for waiting point approximation 19 National Superconducting Cyclotron Laboratory at Michigan State University New Coupled Cyclotron Facility – experiments since mid 2001 Ion Source: 86Kr beam 86Kr beam 140 MeV/u 86Kr hits Be target and fragments Tracking (=Momentum) TOF start Separated beam of r-process nuclei TOF stop dE detector Implant beam in detector and observe decay Fast beam fragmentation facility – allows event by event particle identification 20 H. Schatz NSCL Coupled Cyclotron Facility W. Benenson (NSCL) and B. Richards (WKAR) 21 Installation of D4 steel, Jul/2000 22 First r-process experiments at new NSCL CCF facility (June 02) Measure: • b-decay half-lives • Branchings for b-delayed n-emission Detect: • Particle type (TOF, dE, p) • Implantation time and location • b-emission time and location • neutron-b coincidences New NSCL Neutron detector NERO 3He + n -> t + p neutron Fast Fragment Beam Si Stack (fragment. 140 MeV/u 86Kr) 23 NSCL BCS – Beta Counting System • • • 4 cm x 4 cm active area 1 mm thick 40-strip pitch in x and y dimensions ->1600 pixels Si BCS Si Si b 24 NERO – Neutron Emission Ratio Observer 3He Proportional Counters BF3 Proportional Counters Specifications: • 60 counters total (16 3He , 44 BF3) • 60 cm x 60 cm x 80 cm polyethylene block • Extensive exterior shielding • 43% total neutron efficiency (MCNP) Polyethylene Moderator Boron Carbide Shielding 25 NERO Assembly 26 Nero efficiency NERO Efficiency vs. Neutron Energy Efficiency (%) 50 13C 40 11B 30 20 51V 10 252Cf 0 0.001 0.01 0.1 1 Neutron Energy (MeV) 10 Scaled MCNP Curve 27 Energy loss in Si (Z) Particle Identification Fast RIB from fragmentation: • no decay losses • any beam can be produced • multiple measurements in one • high sensitivity r-process nuclei 78Ni Doubly Magic ! 78Ni 75Co 77Ni 74Co 73Co Time of flight (m/q) 28 H. Schatz Decay data time (ms) time (ms) time (ms) Fast radioactive beams: • No decay losses • Rates as low as 1/day useful ! • Mixed beam experiments easy 29 Results for the main goal: 78Ni (14 neutrons added to stable Ni) Decay of 78Ni : major bottle-neck for synthesis of heavy elements in the r-process Managed to create 11 of the doubly magic 78Ni nuclei in ~ 5 days Time between arrival and decays: Statistical Analysis Result for half-life: 110 +100-60 ms Compare to theoretical estimate used:470 ms time (ms) Acceleration of the entire r-process Models need to be adjusted to explain observed abundance distribution 30 Neutron Data With neutron in addition Nuclei with decay detected 420 420 370 DE (arb units) DE (arb units) Nn 320 76Ni 270 220 350 73Co 400 450 500 550 TOF (arb units) Nn Pn Nb n 370 320 76Ni 270 220 350 73Co 400 450 500 550 TOF (arb units) neutron detection efficiency (neutrons seen/neutrons emitted) 31 Results (Hosmer et al.) DF+CQRPA Borzov et al. 2005, QRPA: Moller et al. 2003, Shell model: Lisetzky & Brown 2005 T1/2 (s) A A Preliminary Pn (%) Preliminary A 32 A H. Schatz Impact of 78Ni half-life on r-process models Observed Solar Abundances 1.E+02 Abundance (A.U.) Model Calculation: Half-Lives from Moeller, et al. 97 Series4 Same but with present 78Ni Result 1.E+01 1.E+00 1.E-01 1.E-02 70 120 170 220 Mass (A) need to readjust r-process model parameters Can obtain Experimental constraints for r-process models from observations and solid nuclear physics remainig discrepancies – nuclear physics ? Environment ? Neutrinos ? Need more data 33 NSCL and future facilities reach Bright future for experiments and observations Experimental test of r-process models is within reach Known half-life Vision: r-process as precision probe NSCL reach Reach of future facility (here: ISF - NSCL upgrade under discussion) 112Mo Mo 111Nb Nb Zr Y 108Zr J. Pereira: (NSCL) 105Y Sr Rb 34 Towards an experimental nuclear physics basis for the r-process Final isotopes, for which >90% of progenitors in the r-process path can be reached experimentally for at least a half-life measurement today Existing facilities ISF These abundances can be compared with observations to test r-process models 35 H. Schatz Collaboration 78Ni Collaboration MSU: P. Hosmer R.R.C. Clement A. Estrade P.F. Mantica F. Montes C. Morton W.F. Mueller E. Pellegrini P. Santi H. Schatz M. Steiner A. Stolz B.E. Tomlin M. Ouellette Mainz: O. Arndt K.-L. Kratz B. Pfeiffer Pacific Northwest Natl. Lab. P. Reeder Notre Dame: A. Aprahamian A. Woehr Maryland: W.B. Walters 36 Overview of common r process models • Site independent models: • nn, T, t parametrization (neutron density, temperature, irradiation time) • S, Ye, t parametrization (Entropy, electron fraction, expansion timescale) • Core collapse supernovae • Neutrino wind • Jets • Explosive helium burning • Neutron star mergers 37 Site independent approach Goal: Use abundance observations as general constraints on r-process conditions BUT: need nuclear physics to do it nn, T, t parametrization (see Prof. K.-L. Kratz transparencies) obtain r-process conditions needed for which the right N=50 and N=82 isotopes are waiting points (A~80 and 130 respectively) often in waiting point approximation Kratz et al. ApJ403(1993)216 38 S, Ye, t parametrization 1. 2. 3. Consider a blob of matter with entropy S, electron abundance Ye in NSE Expand adiabatically with expansion timescale t Calculate abundances - what will happen: 1. 2. 3. 4. NSE QSE (2 clusters: p,n,a and heavy nuclei) a-rich freezeout (for higher S) (3a and aan reactions slowly move matter from p,n,a cluster to heavier nuclei – once a heavy nucleus is created it rapidly captures a-particles as a result large amounts of A~90-100 nuclei are produce which serve as seed for the r-process r-process phase initially: n,g – g,n equilibrium later: freezeout 39 Evolution of equilibria: from Brad Meyers website cross : most abundant nucleus colors: degree of equilibrium with that nucleus (difference in chemical potential) 40 Results for neutron to seed ratios: (Meyer & Brown ApJS112(1997)199) n/seed is higher for • lower Ye (more neutrons) • higher entropy (more light particles, less heavy nuclei – less seeds) (or: low density – low 3a rate – slow seed assembly) • faster expansion (less time to assemble seeds) 2 possible scenarios: 1) high S, moderate Ye 2) low S, low Ye 41 Matter evaporated off the hot neutron star Neutron star forms (size ~ 10 km radius) r-process site ? 42 How does the r-process work ? Neutron capture ! 43 r-process in Supernovae ? Most favored scenario for high entropy: Neutrino heated wind evaporating from proto neutron star in core collapse ne neutrino sphere (ne+p n+e+ weak opacity because only few protons present) ne neutrino sphere (ve+n p+e+ strong opacity because many neutrons present) proto neutron star (n-rich) weak interactions regulate n/p ratio: ne+p n+e+ ne+n p+e- faster as ne come from deeper and are therefore hotter ! therefore matter is driven neutron rich 44 Results for Supernova r-process Takahashi, Witti, & Janka A&A 286(1994)857 (for latest treatment of this scenario see Thompson, Burrows, Meyer ApJ 562 (2001) 887) A~90 overproduction density artificially reduced by factor 5.5 can’t produce A~195 anymore density artificially reduced by factor 5 artificial parameter to get A~195 peak (need S increase) other problem: the a effect 45 other problem: the a effect Recall equilibrium of nucleons in neutrino wind: ne+p n+e+ ne+n p+e- Maintains a slight neutron excess np n p nn 0.4 What happens when a-particles form, leaving a mix of a-particles and neutrons ? 46 r-process in neutron star mergers ? 47 Ejection of matter in NS-mergers Rosswog et al. A&A 341 (1999) 499 Destiny of Matter: red: ejected blue: tails green: disk black: black hole (here, neutron stars are co-rotating – tidally locked) 48 r-process in NS-mergers large neutron/seed ratios, fission cycling ! But: Ye free parameter … 49 Summary theoretical scenarios NS-mergers Supernovae 1e-5 - 1e-4 2.2e-2 Ejected r-process mass (solar masses) 4e-3 – 4e-2 1e-6 – 1e-5 Summary less frequent but more ejection more frequent and less ejection Frequency (per yr and Galaxy) 50 What does galactic chemical evolution observations tell us ? Argast et al. A&A 416 (2004) 997 Supernovae NS mergers Model star average with error observations Average ISM Dots: model stars Neutron Star Mergers ruled out as major contributor 51 r- and s-process elements in stars with varying metallicity (Burris et al. ApJ 544 (2000) 302) s-process: • later (lower mass stars) • gradual onset (range of stars) s-process r-process r-process: • very early (massive stars) • sudden onset (no low mass star contribution) ~age confirms massive stars as r-process sites (but includes SN and NS-mergers) 52 Multiple “r-processes” Star to star stability of all elements (for very r-rich stars) Star to star scatter of light vs heavy for all stars [Fe/H]<-2.5, no s-process (J.J. Cowan) (Honda et al. 2004) Additional “light” element primary process (LEPP) exists (Travaglio et al. 2004 , Montes et al. 2006 to be published) It contributes to solar r-process residual abundances 53 Honda et al. 2006 Ivans et al. 2006 54 Honda et al. 2006 55 56 Disentangling by isotope? 57 58